Two nations are now just 90 minutes away from securing a place in the Euro 2024 final following Friday's action.
Spain were the first to secure their place in the last four of the tournament, as Germany became the first hosts of a European Championship to be eliminated at the quarter-final stage.
Later on, France needed penalties to edge past Portugal, and they will meet Luis de la Fuente's side in Munich.
After another enthralling day of knockout football, we take a deep dive into the best statistics from the day.
Spain 2-1 Germany (AET): Merino's late, late show keeps Spain perfect
Mikel Merino proved to be the hero for Spain as his first international goal got them over the line.
The Real Sociedad midfielder broke German hearts, netting the third-latest winning goal in a European Championship match (118:52), after Michel Platini for France v Portugal at Euro 1984 (118:53) and Artem Dovbyk for Ukraine v Sweden at Euro 2020 (120:36).
While Merino grabbed the headlines, the influential performance of Dani Olmo should not be overlooked.
Olmo replaced Pedri early on in Stuttgart, making his mark in the 51st minute as he steered the ball home after being set up by Lamine Yamal, who became the first teenager to record three assists at a single edition of the Euros (all-time) or World Cup (on record, since 1966).
La Roja's number 10 has made an impact from the bench and is the first Spaniard to score two goals as a substitute at a single edition of the Euros, and the third at any major tournament after Fernando Morientes at the 2002 World Cup and Alvaro Morata at the 2022 World Cup.
Olmo also registered the joint-most shots (three) alongside fellow substitute Mikel Oyarzabal, and only second behind Fabian Ruiz (24) for passes in the final third with 23.
De la Fuente's side roll on to their semi-final clash with France yet to lose at the tournament so far; they are only the third nation to win five in a row during a single edition of the finals (excluding shootouts), after Les Bleus at Euro 1984 and Italy at Euro 2020, both of whom won those respective tournaments.
For Germany, however, their woes in the latter stages of the European Championships continued.
Germany have now lost three of their last four knockout stage games at the Euros (W1), as many as in their previous 12 at the finals beforehand.
Portugal 0-0 France (AET, 3-5 pens): Joao Felix flounders, Ronaldo crashes out
Joao Felix was the unlucky man to fall victim to the lottery of a penalty shootout, with his missed spot-kick allowing Theo Hernandez to set up a meeting with Spain in the semi-finals of Euro 2024.
It will be France's sixth appearance at this stage of the competition, with Didier Deschamps' serial winners only bettered by Germany (eight) for semi-final appearances at the European Championships.
Four of the five European Championship meetings between France and Portugal have now gone beyond the 90 minutes – the only fixture in the tournament’s history to go the distance more than twice.
Despite the plethora of goal-scoring talents both nations have possessed over the years, the encounter in Hamburg was the second Euros game on record (from 1980) not to see a single shot from inside either box in the first half – the other was also France v Portugal in the 1984 semi-final.
Portugal have now gone three games without scoring a goal for the first time since a run of four from December 1996 to March 1997.
Excluding penalties and own goals, France are yet to score in their five games at Euro 2024. No side has ever gone longer without such a goal in the tournament's history, with Les Bleus attempting 86 non-penalty shots (7.25 non-pen xG) without scoring from one at this year’s finals.
Deschamps now has four days to rectify his misfiring strike force, and was given food for thought with the introduction of Ousmane Dembele with 20 minutes to go.
Dembele created more chances (six) than any other player in this match. The only other player to create as many after coming on from the bench in a Euros game on record (since 1980) was Cesc Fabregas for Spain v Russia in 2008 (also six).
For Cristiano Ronaldo, his dreams of closing the curtain on a phenomenal international career with a second honour for his country were shattered in the most gut-wrenching circumstances.
He had 23 shots across the tournament, but failed to score with any of them.
Hurtig the hero after late goal sends Arsenal into Champions League quarters
Lina Hurtig's 89th minute winner ensured Arsenal progressed to the quarter-finals of the Women's Champions League after edging Juventus 1-0 on Thursday.
After being frustrated for large parts of the encounter, Hurtig bundled home from close range after Martina Lenzini's poor clearance to book the Gunners' place in the last eight.
Despite Arsenal dominating the early exchanges, it was Juventus who had the first sight of goal, though Eva Schatzer's effort was easy for Daphne van Domselaar to gather.
In a first half that saw just two shots on target, both coming from the visitors, Renee Slegers' substitutes proved to be the difference for Arsenal.
Slegers introduced Beth Mead, Stina Blackstenius and Hurtig late on, with the latter somehow putting Kim Little's cross over the bar from five yards out.
However, the Swede would atone for her earlier error, combining with fellow substitute Blackstenius to net against her former club and send them out of the competition with two group games remaining.
Meanwhile, in Group D, Barcelona edged closer to the quarter-finals of the competition with a convincing 4-1 victory over St. Polten at the Generali Arena.
The reigning champions are still three points behind Manchester City following their 2-1 win over Hammarby, and know a win against the Swedes next month will see them progress.
Kika Nazareth opened the scoring in the 20th minute after capitalising on a mistake by Kamila Dubcova, notching her second nine minutes later from close range.
Barca found themselves three goals up at the break when Vicky Lopez netted her first goal in the competition to put the result beyond doubt.
There was also a landmark moment for Alexia Putellas, who netted her 200th goal for the club with a well-taken effort into the far corner.
Valentina Madl took some of the shine off an otherwise impressive display from the visitors, who have now taken their tally to 20 goals from their four matches in the competition.
Guardiola agrees two-year contract extension with Man City
Pep Guardiola will be Manchester City manager for at least two more seasons after 2024-25, after he signed a two-year contract extension on Thursday.
The 53-year-old was coming to the end of his City deal, which was due to expire at the end of the current campaign, but he has opted to remain at the Etihad Stadium.
The deal itself will take Guardiola's tenure at the club to over a decade, making him City's longest-serving manager since Les McDowall in 1963.
There had been suggestions that he may leave at the end of the season following the announcement that director of football Txiki Begiristain was on his way out.
Guardiola was strongly linked with the England job after Gareth Southgate resigned in the wake of their Euro 2024 final defeat, but the Football Association appointed Thomas Tuchel last month.
“Manchester City means so much to me," Guardiola said. “This is my ninth season here; we have experienced so many amazing times together. I have a really special feeling for this football club.
“That is why I am so happy to be staying for another two more seasons.
“Thank you to everyone for continuing to trust and support me – The Owner, The Chairman Khaldoon, Ferran, Txiki, the players and, of course, the fans… everyone connected to Manchester City. It has always been an honour, a pleasure and a privilege to be here.
“I have said this many times before, but I have everything a manager could ever wish for, and I appreciate that so much.
“Hopefully, now we can add more trophies to the ones we have already won. That will be my focus.”
Having been appointed in 2016, Guardiola is by some distance Manchester City's most successful manager of all time, having won 18 major trophies during his time at the club.
That list includes their first-ever Champions League triumph in 2023 and six Premier League titles, including an unprecedented four on the spin.
He also boasts a 72.04% win percentage across all competitions, which is unsurprisingly the highest of any full-time City manager in history.
Shaw at the double as Man City progress in Champions League
Khadija Shaw scored twice as Manchester City beat Hammarby 2-1 to seal their place in the Women's Champions League quarter-finals.
Gareth Taylor's team entered Thursday's game with a perfect record in Group D, and their fourth win in as many European matches ensured they finished in the top two.
Shaw—the leading scorer in the Women's Super League this season with eight goals—put them ahead in the 31st minute, driving into the area after taking in Yui Hasegawa's pass before seeing her shot deflect into the top corner.
Shaw was booked for celebrating in front of the home fans despite appearing to have objects thrown at her from the stands, and Hammarby should have levelled when Julia Blakstad fired wide 10 minutes later.
The hosts did draw level three minutes into the second half as Ellen Wangerheim tapped home while City's Laura Blindkilde Brown was down appealing for a free-kick.
That parity was short-lived, though, as Shaw blasted into the top corner from 25 yards out, taking her overall tally for this season to 12 goals in all competitions.
In Group C, meanwhile, Bayern Munich lost their perfect record as they played out a 1-1 draw with Valerenga, boosting Arsenal's hopes of topping the pile.
Jovana Damnjanovic came off the bench to put Bayern ahead 15 minutes from time in Norway, but Elise Thorsnes headed home following an 88th-minute corner to snatch a point for the hosts.
Arsenal could now move within a point of Bayern when they face Juventus in Group C's other match later on Thursday.
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