Ronald Koeman promised Barcelona would "go with everything we have" to secure the LaLiga title on an evening when Atletico Madrid faltered again.
The trophy, and a domestic double, looked unlikely prospects as Barcelona stumbled through the opening months of the season.
Yet they will head into May with the Copa del Rey locked away in the trophy room and league glory could follow.
Long-time leaders Atletico have struggled without former Barcelona frontman Luis Suarez recently, and although he came off the bench in Sunday's clash with Athletic Bilbao, Diego Simeone's wobbling side suffered a 2-1 defeat.
It means that although Atletico still hold a two-point lead at the top, Barcelona and Real Madrid are the closest chasing sides, level on 71 points. Importantly, Barca have a game in hand over both their rivals.
The Camp Nou club's 2-1 win over Villarreal strengthened their championship case, with Real Madrid only able to draw 0-0 with Real Betis on Saturday.
Asked about the prospect of a league and cup double, Koeman said on Sunday: "I have never said that it is impossible, but when you have a distance of points and you are behind, you have to go game by game.
"We're in there. But the best way to win this league is to go game by game."
Speaking after Barcelona's win but before Atletico fell to their jolting defeat, Koeman praised his side, who have now gathered 46 points from a possible 51 since the turn of the year in LaLiga.
Of their last 24 clashes with Villarreal in LaLiga, Barca have won 18 times and drawn the other six, a staggeringly good record against one of Spain's better club sides.
"It is closer, but I don't know if it is very close," Koeman said of the title. "We have a track record of many victories. And what the team are doing is something very big, trying to win LaLiga as well.
"We know that if we win all six games we will be champions. We are going to go with everything we have to try to win LaLiga."
Atletico have lost two of their last five LaLiga games, showing fallibility at just the wrong time. They had previously lost just two of 44 league matches, including a strong finish to last season.
A Camp Nou clash between Atletico and Barcelona on May 8 is the standout fixture of the title run-in, and momentum can quickly turn.
Before that, Barca have games against Granada on Thursday and at Valencia on Sunday.
Koeman said it is "difficult to be 100 per cent" when games are coming so thick and fast.
But having come so far, making up so much ground when at one point qualifying for the Champions League looked to be in doubt, Barcelona are determined not to slow down.
As goalkeeper Marc-Andre ter Stegen put it on Instagram: "6 finals to go. We must be ready for Thursday."
Hurtig the hero after late goal sends Arsenal into Champions League quarters
Lina Hurtig's 89th minute winner ensured Arsenal progressed to the quarter-finals of the Women's Champions League after edging Juventus 1-0 on Thursday.
After being frustrated for large parts of the encounter, Hurtig bundled home from close range after Martina Lenzini's poor clearance to book the Gunners' place in the last eight.
Despite Arsenal dominating the early exchanges, it was Juventus who had the first sight of goal, though Eva Schatzer's effort was easy for Daphne van Domselaar to gather.
In a first half that saw just two shots on target, both coming from the visitors, Renee Slegers' substitutes proved to be the difference for Arsenal.
Slegers introduced Beth Mead, Stina Blackstenius and Hurtig late on, with the latter somehow putting Kim Little's cross over the bar from five yards out.
However, the Swede would atone for her earlier error, combining with fellow substitute Blackstenius to net against her former club and send them out of the competition with two group games remaining.
Meanwhile, in Group D, Barcelona edged closer to the quarter-finals of the competition with a convincing 4-1 victory over St. Polten at the Generali Arena.
The reigning champions are still three points behind Manchester City following their 2-1 win over Hammarby, and know a win against the Swedes next month will see them progress.
Kika Nazareth opened the scoring in the 20th minute after capitalising on a mistake by Kamila Dubcova, notching her second nine minutes later from close range.
Barca found themselves three goals up at the break when Vicky Lopez netted her first goal in the competition to put the result beyond doubt.
There was also a landmark moment for Alexia Putellas, who netted her 200th goal for the club with a well-taken effort into the far corner.
Valentina Madl took some of the shine off an otherwise impressive display from the visitors, who have now taken their tally to 20 goals from their four matches in the competition.
Guardiola agrees two-year contract extension with Man City
Pep Guardiola will be Manchester City manager for at least two more seasons after 2024-25, after he signed a two-year contract extension on Thursday.
The 53-year-old was coming to the end of his City deal, which was due to expire at the end of the current campaign, but he has opted to remain at the Etihad Stadium.
The deal itself will take Guardiola's tenure at the club to over a decade, making him City's longest-serving manager since Les McDowall in 1963.
There had been suggestions that he may leave at the end of the season following the announcement that director of football Txiki Begiristain was on his way out.
Guardiola was strongly linked with the England job after Gareth Southgate resigned in the wake of their Euro 2024 final defeat, but the Football Association appointed Thomas Tuchel last month.
“Manchester City means so much to me," Guardiola said. “This is my ninth season here; we have experienced so many amazing times together. I have a really special feeling for this football club.
“That is why I am so happy to be staying for another two more seasons.
“Thank you to everyone for continuing to trust and support me – The Owner, The Chairman Khaldoon, Ferran, Txiki, the players and, of course, the fans… everyone connected to Manchester City. It has always been an honour, a pleasure and a privilege to be here.
“I have said this many times before, but I have everything a manager could ever wish for, and I appreciate that so much.
“Hopefully, now we can add more trophies to the ones we have already won. That will be my focus.”
Having been appointed in 2016, Guardiola is by some distance Manchester City's most successful manager of all time, having won 18 major trophies during his time at the club.
That list includes their first-ever Champions League triumph in 2023 and six Premier League titles, including an unprecedented four on the spin.
He also boasts a 72.04% win percentage across all competitions, which is unsurprisingly the highest of any full-time City manager in history.
Shaw at the double as Man City progress in Champions League
Khadija Shaw scored twice as Manchester City beat Hammarby 2-1 to seal their place in the Women's Champions League quarter-finals.
Gareth Taylor's team entered Thursday's game with a perfect record in Group D, and their fourth win in as many European matches ensured they finished in the top two.
Shaw—the leading scorer in the Women's Super League this season with eight goals—put them ahead in the 31st minute, driving into the area after taking in Yui Hasegawa's pass before seeing her shot deflect into the top corner.
Shaw was booked for celebrating in front of the home fans despite appearing to have objects thrown at her from the stands, and Hammarby should have levelled when Julia Blakstad fired wide 10 minutes later.
The hosts did draw level three minutes into the second half as Ellen Wangerheim tapped home while City's Laura Blindkilde Brown was down appealing for a free-kick.
That parity was short-lived, though, as Shaw blasted into the top corner from 25 yards out, taking her overall tally for this season to 12 goals in all competitions.
In Group C, meanwhile, Bayern Munich lost their perfect record as they played out a 1-1 draw with Valerenga, boosting Arsenal's hopes of topping the pile.
Jovana Damnjanovic came off the bench to put Bayern ahead 15 minutes from time in Norway, but Elise Thorsnes headed home following an 88th-minute corner to snatch a point for the hosts.
Arsenal could now move within a point of Bayern when they face Juventus in Group C's other match later on Thursday.
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